Molecular Organometallic Materials for Optics


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With the success of this early-late association, we also explored late-late metal bimetallic complexes. Gold-platinum derivatives were thus synthesized using a ditopic phosphine-bipyridylamine assembling ligand Fig.


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  5. Their cytotoxicity on cancer cells was found to be in the range of the one of cisplatin or higher, correlating well with their uptake in cells. Nonetheless, no DNA-adduct could be detected, thus suggesting a different mode of action than cisplatin. We have also developped the synthesis of a NHC ligand bearing an activatable ester that allows its linkage to other ligand-types like phosphines. Using this strategy, homobimetallic gold complexes and heterobimetallic gold-ruthenium and gold-copper complexes were obtained with in vitro antiproliferative properties up to 25 times higher than their monometallic counterpart Fig.

    Taking advantage of our experience in the synthesis of NHC-complexes, we have also designed and studied cafeine- or more generally xanthine-derived NHC monometallic gold complexes Fig. Although exhibiting moderate cytotoxicity on cancer cells, they nonetheless revealed a noteworthy high selectivity, with some of them being almost non toxic on healthy cells and ex vivo precision cut tissue slices collaboration with the University of Groningen, A.

    In collaboration with the universities of Sassari A. Cinellu and Groningen A. Casini , other carbon-gold bond containing complexes were studied Fig. Figure 2. Examples of potential anticancer agents developped in our group. Synthesis and study of biological activities of trans -resveratrol derivatives. The main objective of this work is to investigate the dynamics of both charge and energy transport in these materials. Collaborations with other institutions involve the use of pulse radiolytic and femtosecond transient absorption techniques to better understand migration dynamics.

    We study the properties of aggregates or gels consisting of metal-organic or organometallic-conjugated oligomers or polymers. The primary objective of this project is to design metal-containing molecular arrays that self-assemble in solution and to study the triplet exciton migration on these aggregates. Figure 1 shows a few examples of Platinum-acetylide oligomers which aggregate or gel in hydrocarbon solvents. The molecules stack to form a ordered fibrous network as shown in the TEM images.

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